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Mattan, K.*; Ono, Toshio*; Kawamura, Seiko; Nakajima, Kenji; Nambu, Yusuke*; Sato, Taku*
Physical Review B, 105(13), p.134403_1 - 134403_8, 2022/04
Times Cited Count:3 Percentile:45.85(Materials Science, Multidisciplinary)Spin dynamics of the spin-1/2 kagome-lattice antiferromagnet CsCuSnF was studied using high-resolution, time-of-flight inelastic neutron scattering. The flat mode, a characteristic of the frustrated kagome antiferromagnet, and the low-energy dispersive mode, which is dominated by magnons, can be well described by the linear spin-wave theory. However, the theory fails to describe three weakly dispersive modes between 9 and 14 meV. These modes could be attributed to two-spinon bound states, which decay into free spinons away from the zone center and at a high temperature, giving rise to continuum scattering.
Takeda, Masayasu
Bunseki, 2021(11), p.611 - 615, 2021/11
no abstracts in English
Wu, P.*; Fan, F.-R.*; Hagihara, Masato*; Kofu, Maiko; Peng, K.*; Ishikawa, Yoshihisa*; Lee, S.*; Honda, Takashi*; Yonemura, Masao*; Ikeda, Kazutaka*; et al.
New Journal of Physics (Internet), 22(8), p.083083_1 - 083083_9, 2020/08
Times Cited Count:9 Percentile:57.85(Physics, Multidisciplinary)Thermoelectric material SnSe has aroused world-wide interests in the past years, and its inherent strong lattice anharmonicity is regarded as a crucial factor for its outstanding thermoelectric performance. However, the understanding of lattice anharmonicity in SnSe system remains inadequate, especially regarding how phonon dynamics are affected by this behavior. In this work, we present a comprehensive study of lattice dynamics on NaSnSeS by means of neutron total scattering, inelastic neutron scattering, Raman spectroscopy as well as frozen-phonon calculations. Lattice anharmonicity is evidenced by pair distribution function, inelastic neutron scattering and Raman measurements. By separating the effects of thermal expansion and multi-phonon scattering, we found that the latter is very significant in high-energy optical phonon modes. The strong temperature-dependence of these phonon modes indicate the anharmonicity in this system. Moreover, our data reveals that the linewidths of high-energy optical phonons become broadened with mild doping of sulfur. Our studies suggest that the thermoelectric performance of SnSe could be further enhanced by reducing the contributions of high-energy optical phonon modes to the lattice thermal conductivity via phonon engineering.
Iida, Kazuki*; Yoshida, Hiroyuki*; Nakao, Akiko*; Jeschke, H. O.*; Iqbal, Y.*; Nakajima, Kenji; Kawamura, Seiko; Munakata, Koji*; Inamura, Yasuhiro; Murai, Naoki; et al.
Physical Review B, 101(22), p.220408_1 - 220408_6, 2020/06
Times Cited Count:22 Percentile:80.82(Materials Science, Multidisciplinary)Crystal and magnetic structures of the mineral centennialite CaCu(OD)Cl 0.6DO are investigated by means of synchrotron X-ray diffraction and neutron diffraction measurements complemented by density functional theory (DFT) and pseudofermion functional renormalization group (PFFRG) calculations. In CaCu(OD)Cl 0.6DO, Cu ions form a geometrically perfect kagome network with antiferromagnetic . No intersite disorder between Cu and Ca ions is detected. CaCu(OD)Cl 0.6DO enters a magnetic long-range ordered state below = 7.2 K, and the =0 magnetic structure with negative vector spin chirality is obtained. The ordered moment at 0.3 K is suppressed to 0.58(2)B. Our DFT calculations indicate the presence of antiferromagnetic and ferromagnetic superexchange couplings of a strength which places the system at the crossroads of three magnetic orders (at the classical level) and a spin- PFFRG analysis shows a dominance of =0 type magnetic correlations, consistent with and indicating proximity to the observed =0 spin structure. The results suggest that this material is located close to a quantum critical point and is a good realization of a -- kagome antiferromagnet.
Oi, Motoki
Shiki, 43, P. 3, 2019/06
At the J-PARC Materials and Life Science Facility (MLF), we developed an Au-In-Cd alloy as a low activation neutron absorber for reducing the activity of moderator assembly, and put it to practical use in the reflector and moderator. As a method to confirm the distribution of indium in the alloy, pulse neutron imaging method is adopted, and the individual element distribution is measured by focusing on the resonance peak of indium, and the uniformity of the alloy is confirmed.
Sugiyama, Masaaki*; Nakagawa, Hiroshi; Inoue, Rintaro*; Kawakita, Yukinobu
JAEA-Review 2017-024, 40 Pages, 2017/12
Now-a-days, promotion of life science by utilizing neutron (neutrons biology) is highly demanded in our country, following installation and improvement of high quality and intensity neutron sources at J-PARC and JRR-3. Aiming at accelerating development of neutrons biology in our country, an international workshop "Neutron biology for next generation" was held as a J-PARC Workshop at Ibaraki Quantum Beam Research Center from 22 March to 23 March in 2017. In the workshop, latest instruments, new-fashioned methodologies, recent scientific results and future perspectives were extensively discussed by domestic neutron instrumental scientists and domestic/foreign neutron biologists. This is a report of the workshop summarized by organizers.
Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.
Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12
The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.
Sakasai, Kaoru; Sato, Setsuo*; Seya, Tomohiro*; Nakamura, Tatsuya; To, Kentaro; Yamagishi, Hideshi*; Soyama, Kazuhiko; Yamazaki, Dai; Maruyama, Ryuji; Oku, Takayuki; et al.
Quantum Beam Science (Internet), 1(2), p.10_1 - 10_35, 2017/09
Neutron devices such as neutron detectors, optical devices including supermirror devices and He neutron spin filters, and choppers are successfully developed and installed at the Materials Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), Tokai, Japan. Four software components of MLF computational environment, instrument control, data acquisition, data analysis, and a database, have been developed and equipped at MLF. MLF also provides a wide variety of sample environment options including high and low temperatures, high magnetic fields, and high pressures. This paper describes the current status of neutron devices, computational and sample environments at MLF.
Aso, Tomokazu; Teshigawara, Makoto; Hasegawa, Shoichi; Aoyagi, Katsuhiro*; Muto, Hideki*; Nomura, Kazutaka*; Takada, Hiroshi; Ikeda, Yujiro
JAEA-Technology 2017-021, 75 Pages, 2017/08
Liquid hydrogen is employed as a cold neutron moderator material at the spallation neutron source of Materials and Life science experimental Facility of Japan Proton Accelerator Research Complex (J-PARC). From January 2015, it became observable that the differential pressure between heat exchangers and an 80 K adsorber (ADS) in a helium refrigerator system increased with operating time. In November 2015, the differential pressure rise became more significant, leading to degrade the refrigerating performance in cooling liquid hydrogen. In order to investigate the cause of the abnormal differential pressure rise between the heat exchangers and the ADS, we carried out visual inspection inside the heat exchangers and analyzed the impurities contained in the helium gas. Unfortunately, we could not identify the impurities causing the performance degradation, but observed a trace of oil in the inlet piping of the heat exchanger. Based on investigations of the abnormal events occurred in the refrigerators with similar refrigerating capacity at other facilities, we took measures that cleaning the heat exchangers with Freon and replacing the ADS with new one. As a result, the differential pressure rise phenomenon was removed to recover the performance. We have detected oil from the Freon used for cleaning the heat exchangers and at a felt supporting charcoal packed in the ADS. In particular, oil was accumulated in membranous form onto the felt at the entrance side in the ADS. The amount of oil contained in the helium gas was about 10 ppb or so, less than the design value, in the helium refrigerator. However, the oil accumulated onto the felt in the ADS through long operating period may cause abnormal differential pressure rise, leading to the performance degradation of the helium refrigerator. Further study is needed to specify the cause more clearly.
Seto, Hideki; Ito, Shinichi; Yokoo, Tetsuya*; Endo, Hitoshi*; Nakajima, Kenji; Shibata, Kaoru; Kajimoto, Ryoichi; Kawamura, Seiko; Nakamura, Mitsutaka; Kawakita, Yukinobu; et al.
Biochimica et Biophysica Acta; General Subjects, 1861(1), p.3651 - 3660, 2017/01
Times Cited Count:32 Percentile:80.4(Biochemistry & Molecular Biology)J-PARC, Japan Proton Accelerator Research Complex provides short pulse proton beam at a repetition rate 25 Hz and the maximum power is expected to be 1 MW. Materials and Life Science Experimental Facility (MLF) has 23 neutron beam ports and 21 instruments have already been operated or under construction / commissioning. There are 6 inelastic / quasi-elastic neutron scattering spectrometers and the complementary use of these spectrometers will open new insight for life science.
Oh, J.*; Le, M. D.*; Nahm, H.-H.*; Sim, H.*; Jeong, J.*; Perring, T. G.*; Woo, H.*; Nakajima, Kenji; Kawamura, Seiko; Yamani, Z.*; et al.
Nature Communications (Internet), 7, p.13146_1 - 13146_6, 2016/10
Times Cited Count:57 Percentile:86.72(Multidisciplinary Sciences)Magnons and phonons are fundamental quasiparticles in a solid and can be coupled together to form a hybrid quasi-particle. However, detailed experimental studies on the underlying Hamiltonian of this particle are rare for actual materials. Moreover, the anharmonicity of such magnetoelastic excitations remains largely unexplored, although it is essential for a proper understanding of their diverse thermodynamic behaviour and intrinsic zero-temperature decay. Here we show that in non-collinear antiferromagnets, a strong magnon phonon coupling can significantly enhance the anharmonicity, resulting in the creation of magnetoelastic excitations and their spontaneous decay. By measuring the spin waves over the full Brillouin zone and carrying out anharmonic spin wave calculations using a Hamiltonian with an explicit magnon phonon coupling, we have identified a hybrid magnetoelastic mode in (Y,Lu)MnO and quantified its decay rate and the exchange-striction coupling termrequired to produce it.
Matsuo, Tatsuhito; Arata, Toshiaki*; Oda, Toshiro*; Nakajima, Kenji; Kawamura, Seiko; Kikuchi, Tatsuya; Fujiwara, Satoru
Biochemistry and Biophysics Reports (Internet), 6, p.220 - 225, 2016/07
Soda, Minoru*; Homma, Yuki*; Takamizawa, Satoshi*; Kawamura, Seiko; Nakajima, Kenji; Masuda, Takatsugu*
Journal of the Physical Society of Japan, 85(3), p.034717_1 - 034717_9, 2016/03
Times Cited Count:1 Percentile:11.35(Physics, Multidisciplinary)Inelastic neutron scattering experiments are performed on the nanoporous metal complex Cu--1,4-cyclohexanedicarboxylic acid (Cu-CHD) adsorbing O molecules to identify the spin model of the O-based magnet realized in the host complex. It is found that the magnetic excitations of Cu-CHDs adsorbing low- and high-concentration O molecules are explained by different spin models, the former by spin dimers and the latter by spin trimers. By using the obtained parameters and by assuming that the levels of the group of the highest energy states are reduced because of the nonnegligible spin dependence of the molecular potential of oxygen, the magnetization curves are explained quantitatively.
Oi, Motoki; Sakai, Kenji; Watanabe, Akihiko; Akutsu, Atsushi; Meigo, Shinichiro; Takada, Hiroshi
JPS Conference Proceedings (Internet), 8, p.036007_1 - 036007_5, 2015/09
This paper reports on upgrading of the monitor and operation (MO) system for a general control system (GCS) of the Materials and Life science experimental Facility (MLF) at J-PARC. The MLF-GCS consists of programmable logic controllers (PLCs), operator interfaces (OPIs) for integral control and interlock systems, shared servers, and so on. It is controlling various components of the pulsed spallation neutron source such as a mercury target and hydrogen moderators. The MO system is used for monitoring, alarm notification and remote control from the MLF control room. The GCS has been working well as expected, but current MO system which consists of the OPIs and data servers based on iFix has some problems in view of sustainable maintenance because of its poor flexibility of supported OS and software version compatibility. To overcome the problems, we upgraded the MO system to be operated using the framework of EPICS, the OPI of Control System Studio (CSS) and the server software of Postgre SQL. This improves versatility of the MO system, enabling to run on various platforms such as Windows, Linux and Mac OS. At first, we made a prototype MO system, which processed 100 points of data and 5 operation screens and verified that the MO system functions correctly. Then we made full spec MO system which processes the data point of 7000 and operation screens of 130. It was operated in parallel with the current system to evaluate its performance with real data such as data transmission speed from PLCs, control functions from OPI, storage capability of servers and long-term reliability. As results, the new MO system achieved the communication speed of 2 Hz and its operability compatible to the current system. Now, we are operating and debugging it in comparison with the current system during the operating period as a preparation for the system replacement at the end of 2014.
Yamada, Norifumi*; Takeda, Masayasu; Yamazaki, Dai
Hamon, 24(4), p.288 - 295, 2014/11
no abstracts in English
Ikeda, Yujiro
Proceedings of ICANS-XVI, Volume 1, p.13 - 24, 2003/07
no abstracts in English
Yamada, Yasusada*; Watanabe, Noboru*; Niimura, Nobuo; Morii, Yukio; Katano, Susumu; Aizawa, Kazuya; Suzuki, Junichi; Koizumi, Satoshi; Osakabe, Toyotaka; Teshigawara, Makoto*; et al.
Physica B; Condensed Matter, 241-243, p.42 - 45, 1998/00
Times Cited Count:4 Percentile:33.02(Physics, Condensed Matter)no abstracts in English
Yamada, Yasusada*; Watanabe, Noboru*; Niimura, Nobuo*; Morii, Yukio; Katano, Susumu; Aizawa, Kazuya; Suzuki, Junichi; ; Osakabe, Toyotaka
JAERI-Review 96-019, 43 Pages, 1997/01
no abstracts in English
Takeda, Masayasu; Yamazaki, Dai; Soyama, Kazuhiko; To, Kentaro; Yamagishi, Hideshi*; Katagiri, Masaki*; Sakasai, Kaoru; Mizusawa, Tazuko*; Miyata, Noboru*; Kasai, Satoshi*; et al.
no journal, ,
Oi, Motoki; Harada, Masahide; Kai, Tetsuya; Aizawa, Kazuya; Sato, Koichi; Masuyama, Koichi; Kasugai, Yoshimi
no journal, ,
In the J-PARC Materials and Life Science Experimental Facility (MLF), material science experiments using muon and neutron beam are performed. In the MLF, proton beam power was 300KW at May 2014 and it is planning to enhance to 1MW. For proton beam enhancement, we performed evaluation of the shielding performance of the neutron beam instruments. As a result, dose on the shield surface of 16 neutron instruments are sufficiently low for 1MW proton beam operation. However, 4 neutron instruments show high dose rate in particular neutron beam conditions. For these neutron instruments, we have checked the drawings and recalculate the shielding performance and considered a cause. Then based on the measurement results, some shield are added for these four neutron instruments and dose rate are reduced sufficiently to 1MW proton beam operation.